Delay in Photoemission

M. Schultze; M. Fiess; N. Karpowicz; J. Gagnon; M. Korbman; S. Neppl; A. L. Cavalieri; Y. Komninos; Th. Mercouris; C. A. Nicolaides; R. Pazourek; S. Nagele; J. Feist; J. Burgdoerfer; A. M. Azzeer; R. Ernstorfer; R. Kienberger; U. Kleineberg; E. Goulielmakis; F. Krausz; V. S. Yakovlev

doi:10.1126/science.1189401

Delay in Photoemission

M. Schultze, M. Fiess, N. Karpowicz, J. Gagnon, M. Korbman, S. Neppl, A. L. Cavalieri, Y. Komninos, Th. Mercouris, C. A. Nicolaides, R. Pazourek, S. Nagele, J. Feist, J. Burgdoerfer, A. M. Azzeer, R. Ernstorfer, R. Kienberger, U. Kleineberg, E. Goulielmakis, F. KrauszV. S. Yakovlev

Research output: Contribution to journal › Article › peer-review

Abstract

Photoemission from atoms is assumed to occur instantly in response to incident radiation and provides the basis for setting the zero of time in clocking atomic-scale electron motion. We used attosecond metrology to reveal a delay of attoseconds in the emission of electrons liberated from the 2p orbitals of neon atoms with respect to those released from the 2s orbital by the same 100–electron volt light pulse. Small differences in the timing of photoemission from different quantum states provide a probe for modeling many-electron dynamics. Theoretical models refined with the help of attosecond timing metrology may provide insight into electron correlations and allow the setting of the zero of time in atomic-scale chronoscopy with a precision of a few attoseconds.

Original language	English
Pages (from-to)	1658-1662
Journal	Science
Volume	328
Issue number	5986
DOIs	https://doi.org/10.1126/science.1189401
Publication status	Published - 25 Jun 2010
Externally published	Yes

Fields of Expertise

Advanced Materials Science

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10.1126/science.1189401

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Schultze, M., Fiess, M., Karpowicz, N., Gagnon, J., Korbman, M., Neppl, S., Cavalieri, A. L., Komninos, Y., Mercouris, T., Nicolaides, C. A., Pazourek, R., Nagele, S., Feist, J., Burgdoerfer, J., Azzeer, A. M., Ernstorfer, R., Kienberger, R., Kleineberg, U., Goulielmakis, E., ... Yakovlev, V. S. (2010). Delay in Photoemission. Science, 328(5986), 1658-1662. https://doi.org/10.1126/science.1189401

Delay in Photoemission. / Schultze, M.; Fiess, M.; Karpowicz, N.; Gagnon, J.; Korbman, M.; Neppl, S.; Cavalieri, A. L.; Komninos, Y.; Mercouris, Th.; Nicolaides, C. A.; Pazourek, R.; Nagele, S.; Feist, J.; Burgdoerfer, J.; Azzeer, A. M.; Ernstorfer, R.; Kienberger, R.; Kleineberg, U.; Goulielmakis, E.; Krausz, F.; Yakovlev, V. S.

In: Science, Vol. 328, No. 5986, 25.06.2010, p. 1658-1662.

Research output: Contribution to journal › Article › peer-review

Schultze, M, Fiess, M, Karpowicz, N, Gagnon, J, Korbman, M, Neppl, S, Cavalieri, AL, Komninos, Y, Mercouris, T, Nicolaides, CA, Pazourek, R, Nagele, S, Feist, J, Burgdoerfer, J, Azzeer, AM, Ernstorfer, R, Kienberger, R, Kleineberg, U, Goulielmakis, E, Krausz, F & Yakovlev, VS 2010, 'Delay in Photoemission', Science, vol. 328, no. 5986, pp. 1658-1662. https://doi.org/10.1126/science.1189401

Schultze, M. ; Fiess, M. ; Karpowicz, N. ; Gagnon, J. ; Korbman, M. ; Neppl, S. ; Cavalieri, A. L. ; Komninos, Y. ; Mercouris, Th. ; Nicolaides, C. A. ; Pazourek, R. ; Nagele, S. ; Feist, J. ; Burgdoerfer, J. ; Azzeer, A. M. ; Ernstorfer, R. ; Kienberger, R. ; Kleineberg, U. ; Goulielmakis, E. ; Krausz, F. ; Yakovlev, V. S. / Delay in Photoemission. In: Science. 2010 ; Vol. 328, No. 5986. pp. 1658-1662.

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abstract = "Photoemission from atoms is assumed to occur instantly in response to incident radiation and provides the basis for setting the zero of time in clocking atomic-scale electron motion. We used attosecond metrology to reveal a delay of attoseconds in the emission of electrons liberated from the 2p orbitals of neon atoms with respect to those released from the 2s orbital by the same 100–electron volt light pulse. Small differences in the timing of photoemission from different quantum states provide a probe for modeling many-electron dynamics. Theoretical models refined with the help of attosecond timing metrology may provide insight into electron correlations and allow the setting of the zero of time in atomic-scale chronoscopy with a precision of a few attoseconds.",

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AU - Schultze, M.

AU - Fiess, M.

AU - Karpowicz, N.

AU - Gagnon, J.

AU - Korbman, M.

AU - Neppl, S.

AU - Cavalieri, A. L.

AU - Komninos, Y.

AU - Mercouris, Th.

AU - Nicolaides, C. A.

AU - Pazourek, R.

AU - Nagele, S.

AU - Feist, J.

AU - Burgdoerfer, J.

AU - Azzeer, A. M.

AU - Ernstorfer, R.

AU - Kienberger, R.

AU - Kleineberg, U.

AU - Goulielmakis, E.

AU - Krausz, F.

AU - Yakovlev, V. S.

PY - 2010/6/25

Y1 - 2010/6/25

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AB - Photoemission from atoms is assumed to occur instantly in response to incident radiation and provides the basis for setting the zero of time in clocking atomic-scale electron motion. We used attosecond metrology to reveal a delay of attoseconds in the emission of electrons liberated from the 2p orbitals of neon atoms with respect to those released from the 2s orbital by the same 100–electron volt light pulse. Small differences in the timing of photoemission from different quantum states provide a probe for modeling many-electron dynamics. Theoretical models refined with the help of attosecond timing metrology may provide insight into electron correlations and allow the setting of the zero of time in atomic-scale chronoscopy with a precision of a few attoseconds.

U2 - 10.1126/science.1189401

DO - 10.1126/science.1189401

M3 - Article

VL - 328

SP - 1658

EP - 1662

JO - Science

JF - Science

SN - 0036-8075

IS - 5986

ER -

Delay in Photoemission

Abstract

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