Abstract
Original language | English |
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Pages (from-to) | 1601-1610 |
Number of pages | 10 |
Journal | ECS Transactions |
Volume | 91 |
Issue number | 1 |
DOIs | |
Publication status | Published - 1 Sep 2019 |
Event | 16th International Symposium on Solid Oxide Fuel Cells (SOFC-XVI) - Kyoto, Japan Duration: 8 Sep 2019 → 13 Sep 2019 |
Cite this
Ammonia as Promising Fuel for Solid Oxide Fuel Cells: Experimental Analysis and Performance Evaluation. / Stöckl, Bernhard; Preininger, Michael; Subotić, Vanja; Schröttner, Hartmuth; Sommersacher, Peter; Seidl, Michael; Megel, Stefan; Hochenauer, Christoph.
In: ECS Transactions, Vol. 91, No. 1, 01.09.2019, p. 1601-1610.Research output: Contribution to journal › Conference article › Research › peer-review
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TY - JOUR
T1 - Ammonia as Promising Fuel for Solid Oxide Fuel Cells: Experimental Analysis and Performance Evaluation
AU - Stöckl, Bernhard
AU - Preininger, Michael
AU - Subotić, Vanja
AU - Schröttner, Hartmuth
AU - Sommersacher, Peter
AU - Seidl, Michael
AU - Megel, Stefan
AU - Hochenauer, Christoph
PY - 2019/9/1
Y1 - 2019/9/1
N2 - In the course of this study the direct utilization of ammonia in different types of solid oxide fuel cells (SOFCs), such as anode- and electrolyte-supported SOFC, is investigated. Experiments in low fuel utilization, exhibited excellent performance of ammonia in SOFCs, although the power outputs of equivalent hydrogen/nitrogen fuels were not attained due to the incomplete endothermic ammonia decomposition. Next, the single cells were operated under high fuel utilization conditions and methane was added to the humidified ammonia stream, where they showed excellent ammonia- and methane conversions. The stability of the cells used was proven over a period of at least 48 hours with a variety of fuel mixtures. Post mortem scanning electron microscopy analysis of the anode micro-structures indicated nitriding effects of nickel, as microscopic pores and enlargements of the metallic parts occurred. Finally, a long-term test over 1,000 hours was carried out using a ten-layer stack consisting of electrolyte-supported cells.
AB - In the course of this study the direct utilization of ammonia in different types of solid oxide fuel cells (SOFCs), such as anode- and electrolyte-supported SOFC, is investigated. Experiments in low fuel utilization, exhibited excellent performance of ammonia in SOFCs, although the power outputs of equivalent hydrogen/nitrogen fuels were not attained due to the incomplete endothermic ammonia decomposition. Next, the single cells were operated under high fuel utilization conditions and methane was added to the humidified ammonia stream, where they showed excellent ammonia- and methane conversions. The stability of the cells used was proven over a period of at least 48 hours with a variety of fuel mixtures. Post mortem scanning electron microscopy analysis of the anode micro-structures indicated nitriding effects of nickel, as microscopic pores and enlargements of the metallic parts occurred. Finally, a long-term test over 1,000 hours was carried out using a ten-layer stack consisting of electrolyte-supported cells.
U2 - 10.1149/09101.1601ecst
DO - 10.1149/09101.1601ecst
M3 - Conference article
VL - 91
SP - 1601
EP - 1610
JO - ECS Transactions
JF - ECS Transactions
SN - 1938-5862
IS - 1
ER -