Impact ionization processes in the steady state of a driven Mott insulating layer coupled to metallic leads

Max Erich Sorantin, Enrico Arrigoni, Antonius Dorda, Karsten Held

Publikation: Beitrag in einer FachzeitschriftArtikelForschungBegutachtung

Abstract

We study a simple model of photovoltaic energy harvesting across a Mott-insulating gap consisting of a
correlated layer connected to two metallic leads held at different chemical potentials. We address, in particular,
the issue of impact ionization, whereby a particle photoexcited to the high-energy part of the upper Hubbard band
uses its extra energy to produce a second particle-hole excitation. We find a drastic increase of the photocurrent
upon entering the frequency regime where impact ionization is possible. At large values of the Mott gap, where
impact ionization is energetically not allowed, we observe a suppression of the current and a piling up of charge
in the high-energy part of the upper Hubbard band. Our study is based on a Floquet dynamical mean-field theory
treatment of the steady state with the so-called auxiliary master equation approach as impurity solver. We verify
that an additional approximation, taking the self-energy diagonal in the Floquet indices, is appropriate for the
parameter range we are considering.
Originalspracheenglisch
Aufsatznummer115113
Seitenumfang10
FachzeitschriftPhysical Review / B
Jahrgang97
Ausgabenummer11
DOIs
PublikationsstatusVeröffentlicht - 8 Mär 2018

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Impact ionization
ionization
Energy harvesting
Chemical potential
Ionization
Piles
Impurities
energy
retarding
impurities
approximation
excitation

Fields of Expertise

  • Advanced Materials Science

Treatment code (Nähere Zuordnung)

  • Theoretical

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Impact ionization processes in the steady state of a driven Mott insulating layer coupled to metallic leads. / Sorantin, Max Erich; Arrigoni, Enrico; Dorda, Antonius; Held, Karsten.

in: Physical Review / B, Jahrgang 97, Nr. 11, 115113, 08.03.2018.

Publikation: Beitrag in einer FachzeitschriftArtikelForschungBegutachtung

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AB - We study a simple model of photovoltaic energy harvesting across a Mott-insulating gap consisting of acorrelated layer connected to two metallic leads held at different chemical potentials. We address, in particular,the issue of impact ionization, whereby a particle photoexcited to the high-energy part of the upper Hubbard banduses its extra energy to produce a second particle-hole excitation. We find a drastic increase of the photocurrentupon entering the frequency regime where impact ionization is possible. At large values of the Mott gap, whereimpact ionization is energetically not allowed, we observe a suppression of the current and a piling up of chargein the high-energy part of the upper Hubbard band. Our study is based on a Floquet dynamical mean-field theorytreatment of the steady state with the so-called auxiliary master equation approach as impurity solver. We verifythat an additional approximation, taking the self-energy diagonal in the Floquet indices, is appropriate for theparameter range we are considering.

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