Atom-surface van der Waals potentials of topological insulators and semimetals from scattering measurements

Anton Tamtögl*, Adrian Ruckhofer, Davide Campi, William Allison, Wolfgang E Ernst

*Korrespondierende/r Autor/in für diese Arbeit

Publikation: Beitrag in einer FachzeitschriftReview eines Fachbereichs (Review article)

Abstract

The phenomenology of resonant scattering has been known since the earliest experiments upon scattering of atomic beams from surfaces and is a means of obtaining experimental information about the fundamentals of weak adsorption systems in the van der Waals regime. We provide an overview of the experimental approach based on new experimental data for the He-Sb 2Te 3(111) system, followed by a comparative overview and perspective of recent results for topological semimetal and insulator surfaces. Moreover, we shortly discuss the perspectives of calculating helium-surface interaction potentials fromab initiocalculations. Our perspective demonstrates that atom-surface scattering provides direct experimental information about the atom-surface interaction in the weak physisorption regime and can also be used to determine the lifetime and mean free path of the trapped atom. We further discuss the effects of elastic and inelastic scattering on the linewidth and lifetime of the trapped He atom with an outlook on future developments and applications.

Originalspracheenglisch
Seiten (von - bis)7637–7652
Seitenumfang16
FachzeitschriftPhysical Chemistry, Chemical Physics
Jahrgang23
Ausgabenummer13
DOIs
PublikationsstatusVeröffentlicht - 7 Apr 2021

ASJC Scopus subject areas

  • !!Physics and Astronomy(all)
  • !!Physical and Theoretical Chemistry
  • !!Materials Science(all)

Fields of Expertise

  • Advanced Materials Science

Kooperationen

  • NAWI Graz

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